No. This is due to Crunchyroll have separate videos for each audio. You can subscribe to Crunchyroll via Amazon channel (if you're already a Prime member)--Amazon offers multi audio tracks, but the subtitles can be a pain. Or you can download both videos then remux the audio and subtitle into one video using Mkvtoolnix. This only works if both videos have the exact same length (one or the other might have an extra opening, especially older titles)
